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AGU: Geophysical Research Letters

 

Index Terms

  • Atmospheric Composition and Structure: Pollution—urban and regional
  • Atmospheric Composition and Structure: Troposphere—composition and chemistry
  • Global Change: Atmosphere

Abstract

Fresh air in the 21st century?

Michael Prather

Department of Earth System Science, UC Irvine, California, USA

Michael Gauss

Institutt for Geofysikk, University of Oslo, Oslo, Norway

Terje Berntsen

Institutt for Geofysikk, University of Oslo, Oslo, Norway

Ivar Isaksen

Institutt for Geofysikk, University of Oslo, Oslo, Norway

Jostein Sundet

Institutt for Geofysikk, University of Oslo, Oslo, Norway

Isabelle Bey

Swiss Federal Institute of Technology, Lausanne, Switzerland

Guy Brasseur

Max Planck Institute for Meteorology, Hamburg, Germany

Frank Dentener

Joint Research Centre, Environment Institute, Ispra, Italy

Richard Derwent

The Hadley Centre, UK Met Office, Bracknell, United Kingdom

David Stevenson

The Hadley Centre, UK Met Office, Bracknell, United Kingdom

Lee Grenfell

Didier Hauglustaine

Institut Pierre Simon Laplace, CEA-CNRS, Gif-sur-Yvette, France

Larry Horowitz

Geophysical Fluid Dynamics Laboratory, NOAA, Princeton, New Jersey, USA

Daniel Jacob

Dept of Earth & Planetary Sciences, Harvard U., Cambridge, Maryland, USA

Loretta Mickley

Dept of Earth & Planetary Sciences, Harvard U., Cambridge, Maryland, USA

Mark Lawrence

Max Planck Institute for Chemistry, Mainz, Germany

Rolf von Kuhlmann

Max Planck Institute for Chemistry, Mainz, Germany

Jean-Francois Muller

Belgian Institute for Space Aeronomy, Brussels, Belgium

Giovanni Pitari

Dipartimento di Fisica, U.L'Aquila, Coppito, L'Aquila, Italy

Helen Rogers

Centre for Atmos. Sci., Cambridge U., Cambridge, United Kingdom

Matthew Johnson

Centre for Atmos. Sci., Cambridge U., Cambridge, United Kingdom

John Pyle

Centre for Atmos. Sci., Cambridge U., Cambridge, United Kingdom

Kathy Law

Centre for Atmos. Sci., Cambridge U., Cambridge, United Kingdom

Michiel van Weele

Royal Netherlands Meteorological Inst., De Bilt, The Netherlands

Oliver Wild

Frontier Research System for Global Change, Yokohama, Japan

Ozone is an air quality problem today for much of the world's population. Regions can exceed the ozone air quality standards (AQS) through a combination of local emissions, meteorology favoring pollution episodes, and the clean-air baseline levels of ozone upon which pollution builds. The IPCC 2001 assessment studied a range of global emission scenarios and found that all but one projects increases in global tropospheric ozone during the 21st century. By 2030, near-surface increases over much of the northern hemisphere are estimated to be about 5 ppb (+2 to +7 ppb over the range of scenarios). By 2100 the two more extreme scenarios project baseline ozone increases of >20 ppb, while the other four scenarios give changes of −4 to +10 ppb. Even modest increases in the background abundance of tropospheric ozone might defeat current AQS strategies. The larger increases, however, would gravely threaten both urban and rural air quality over most of the northern hemisphere.

Published 31 January 2003.

Citation: Prather, M., et al. (2003), Fresh air in the 21st century?, Geophys. Res. Lett., 30(2), 1100, doi:10.1029/2002GL016285.

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