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JOURNAL OF GEOPHYSICAL RESEARCH,
VOL. 108, NO. D23,
8668,
doi:10.1029/2002JD002845,
2003
Regional chemical weather forecasting system CFORS: Model descriptions and analysis of surface observations at Japanese island
stations during the ACE-Asia experiment
I. Uno
Research Institute for Applied Mechanics, Kyushu University, Kasuga, Japan Frontier Research System for Global Change, Yokohama, Japan
G. R. Carmichael
Center for Global and Regional Environmental Research, University of Iowa, Iowa City, Iowa, USA
D. G. Streets
Argonne National Laboratory, Argonne, Illinois, USA
Y. Tang
Center for Global and Regional Environmental Research, University of Iowa, Iowa City, Iowa, USA
J. J. Yienger
Cities for Climate Protection Campaign, International Council for Local Environmental Initiatives, U.S. Office, Berkeley,
California, USA
S. Satake
Research Institute for Applied Mechanics, Kyushu University, Kasuga, Japan
Z. Wang
Frontier Research System for Global Change, Yokohama, Japan
Jung-Hun Woo
Center for Global and Regional Environmental Research, University of Iowa, Iowa City, Iowa, USA
S. Guttikunda
Center for Global and Regional Environmental Research, University of Iowa, Iowa City, Iowa, USA
M. Uematsu
Ocean Research Institute, University of Tokyo, Tokyo, Japan
K. Matsumoto
Ocean Research Institute, University of Tokyo, Tokyo, Japan Japan Science and Technology Corporation, Tokyo, Japan
H. Tanimoto
National Institute for Environmental Studies, Tsukuba, Japan
K. Yoshioka
Shimane Prefectural Institute of Public Health and Environmental Science, Matsue, Japan
T. Iida
Graduate School of Engineering, Nagoya University, Nagoya, Japan
Abstract
The Chemical Weather Forecast System (CFORS) is designed to aid in the design of field experiments and in the interpretation/postanalysis
of observed data. The system integrates a regional chemical transport model with a multitracer, online system built within
the Regional Atmospheric Modeling System (RAMS) mesoscale model. CFORS was deployed in forecast and postanalysis modes during
the NASA Global Tropospheric Experiment (GTE)-Transport and Chemical Evolution over the Pacific (TRACE-P), International Global
Atmospheric Chemistry project (IGAC)-International Geosphere-Biosphere Programme (IGBP) Asian Pacific Regional Aerosol Characterization
Experiment (ACE-Asia), and National Oceanic and Atmospheric Administration Intercontinental Transport and Chemical Transformation
of Anthropogenic Pollution 2002 (ITCT 2K2) field studies. A description of the CFORS model system is presented. The model
is used to help interpret the Variability of Maritime Aerosol Properties (VMAP) surface observation data. The CFORS model
results help to explain the time variation of both anthropogenic pollutants (sulfate, black carbon, and CO) and natural constituents
including radon and mineral dust. Time series and time-height cross-section analysis of gases and aerosols are presented to
help identify key processes. Synoptic-scale weather changes are found to play an important role in the continental-scale transport
of pollution in the springtime in East Asia. The complex vertical and horizontal structure of pollutants in these outflow
events is also presented and discussed.
Received 14
August
2002;
accepted 17
April
2003;
published 7
August
2003.
Index Terms: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0345 Atmospheric Composition and Structure: Pollution—urban and regional (0305); 0365 Atmospheric Composition and Structure: Troposphere—composition and chemistry.
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Citation: Uno, I., et al.
(2003),
Regional chemical weather forecasting system CFORS: Model descriptions and analysis of surface observations at Japanese island
stations during the ACE-Asia experiment,
J. Geophys. Res.,
108(D23),
8668,
doi:10.1029/2002JD002845.
Copyright 2003 by the American Geophysical Union.
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