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GEOPHYSICAL RESEARCH LETTERS,
VOL. 30, NO. 18,
1936,
doi:10.1029/2003GL017642,
2003
Effect of Climate Change on Isoprene Emissions and Surface Ozone Levels
M. G. Sanderson
Met Office, Bracknell, Berkshire, U.K.
C. D. Jones
Met Office, Bracknell, Berkshire, U.K.
W. J. Collins
Met Office, Bracknell, Berkshire, U.K.
C. E. Johnson
Met Office, Bracknell, Berkshire, U.K.
R. G. Derwent
Met Office, Bracknell, Berkshire, U.K.
Abstract
The effect of climate change on vegetation, isoprene emissions and surface ozone levels was investigated using a global three-dimensional
general circulation model coupled to a dynamic vegetation and chemistry models. Integrations for the 1990s and 2090s were
performed. Isoprene emissions increased from 549 Tg yr−1 (1990s) to 736 Tg yr−1 (2090s) as a result of climate change with fixed vegetation. However, the isoprene emissions only increase to 697 Tg yr−1 in the 2090s when vegetation changes were included. Surface ozone levels rose by 20–30 ppbv in some locations with fixed
vegetation owing to increases in precursor gases, but only by 10–20 ppbv if the vegetation changes were included. Ozone levels
in parts of China, Korea and the eastern USA are predicted to exceed the World Health Organisation health limit of 60 ppbv,
however, when changes in vegetation are accounted for, a much smaller area exceeds this limit.
Received 29
April
2003;
accepted 14
August
2003;
published 20
September
2003.
Index Terms: 0315 Atmospheric Composition and Structure: Biosphere/atmosphere interactions; 0365 Atmospheric Composition and Structure: Troposphere—composition and chemistry; 0325 Atmospheric Composition and Structure: Evolution of the atmosphere; 1610 Global Change: Atmosphere (0315, 0325).
Read Full Article (file size: 82436 bytes) Cited by
Citation: Sanderson, M. G., C. D. Jones, W. J. Collins, C. E. Johnson, and R. G. Derwent
(2003),
Effect of Climate Change on Isoprene Emissions and Surface Ozone Levels,
Geophys. Res. Lett.,
30(18),
1936,
doi:10.1029/2003GL017642.
Published in 2003 by the American Geophysical Union.
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