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AGU: Journal of Geophysical Research, Atmospheres

 

Keywords

  • lidar
  • nephelometer
  • extinction
  • scattering
  • mass scattering
  • Supersite

Index Terms

  • Atmospheric Composition and Structure: Aerosols and particles
  • Atmospheric Composition and Structure: Pollution—urban and regional
  • Atmospheric Composition and Structure: Transmission and scattering of radiation
  • Meteorology and Atmospheric Dynamics: Radiative processes
  • Meteorology and Atmospheric Dynamics: Remote sensing
Abstract
Cited By (5)
 

Abstract

JOURNAL OF GEOPHYSICAL RESEARCH, VOL. 109, D16S02, 15 PP., 2004
doi:10.1029/2003JD004047

Aerosol optical characterization by nephelometer and lidar: The Baltimore Supersite experiment during the Canadian forest fire smoke intrusion

Mariana Adam

Department of Geography and Environmental Engineering, Johns Hopkins University, Baltimore, Maryland, USA

Markus Pahlow

Department of Geography and Environmental Engineering, Johns Hopkins University, Baltimore, Maryland, USA

Vladimir A. Kovalev

Fire Science Laboratory, U.S. Department of Agriculture, Missoula, Montana, USA

John M. Ondov

Department of Chemistry and Biochemistry, University of Maryland, College Park, Maryland, USA

Marc B. Parlange

Department of Geography and Environmental Engineering, Johns Hopkins University, Baltimore, Maryland, USA

Narayanan Nair

Department of Chemistry and Biochemistry, University of Maryland, College Park, Maryland, USA

High spatial and temporal resolution elastic backscatter lidar data from Baltimore are analyzed with a near-end approach to estimate vertical profiles of the aerosol extinction coefficient. The near-end approach makes use of the (1) aerosol scattering coefficient measured at the surface with a nephelometer (0.530 μm), (2) surface level particle size distribution, and (3) refractive index calculated using Mie theory to estimate the aerosol extinction coefficient boundary condition for the lidar equation. There was a broad range of atmospheric turbidity due to a strong haze event, which occurred because of smoke transport from Canadian forest fires, and led to a wide range of observed atmospheric properties. The index of refraction for aerosols estimated during the entire study period is 1.5–0.47 i, which is typical for soot. The measured surface level aerosol scattering coefficient ranged from σ p = 0.002 to σ p = 0.541 km−1, and the computed aerosol extinction coefficient spanned values κ p = 0.01 to κ p = 1.05 km−1. The derived mass concentration and the mass scattering ranges were 3.96–194 μg m−3 and 0.05–3.260 m2g−1, respectively. The aerosol optical properties were dominated by light absorption by soot.

Received 4 August 2003; accepted 20 May 2004; published 21 July 2004.

Citation: Adam, M., M. Pahlow, V. A. Kovalev, J. M. Ondov, M. B. Parlange, and N. Nair (2004), Aerosol optical characterization by nephelometer and lidar: The Baltimore Supersite experiment during the Canadian forest fire smoke intrusion, J. Geophys. Res., 109, D16S02, doi:10.1029/2003JD004047.

Cited By

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