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GEOPHYSICAL RESEARCH LETTERS, VOL. 31, L20506, doi:10.1029/2004GL020915, 2004

Direct observations of the effects of aerosol loading on net ecosystem CO2 exchanges over different landscapes

Dev Niyogi

Department of MEAS, North Carolina State University, Raleigh, North Carolina, USA


Hsin-I Chang

Department of MEAS, North Carolina State University, Raleigh, North Carolina, USA


V. K. Saxena

Department of MEAS, North Carolina State University, Raleigh, North Carolina, USA


Teddy Holt

Department of MEAS, North Carolina State University, Raleigh, North Carolina, USA


Kiran Alapaty

University of North Carolina at Chapel Hill, Raleigh, North Carolina, USA


Fitzgerald Booker

USDA-ARS Air Quality–Plant Growth and Development Unit, Raleigh, North Carolina, USA


Fei Chen

National Center for Atmospheric Research, Boulder, Colorado, USA


Kenneth J. Davis

Department of Meteorology, Pennsylvania State University, University Park, Pennsylvania, USA


Brent Holben

NASA Goddard Space Flight Center, Greenbelt, Maryland, USA


Toshihisa Matsui

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA


Tilden Meyers

Atmospheric Turbulence and Diffusion Division, National Oceanic and Atmospheric Administration, Oak Ridge, Tennessee, USA


Walter C. Oechel

San Diego State University, San Diego, California, USA


Roger A. Pielke Sr.

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA


Randy Wells

Department of Crop Science, North Carolina State University, Raleigh, North Carolina, USA


Kell Wilson

Atmospheric Turbulence and Diffusion Division, National Oceanic and Atmospheric Administration, Oak Ridge, Tennessee, USA


Yongkang Xue

Department of Geography, University of California, Los Angeles, Los Angeles, California, USA


Abstract

We present the first direct, multisite observations in support of the hypothesis that atmospheric aerosols affect the regional terrestrial carbon cycle. The daytime growing season (summer) CO2 flux observations from six sites (forest, grasslands, and croplands) with collocated aerosol and surface radiation measurements were analyzed for high and low diffuse radiation; effect of cloud cover; and effect of high and low aerosol optical depths (AOD). Results indicate that, aerosols exert a significant impact on net CO2 exchange, and their effect may be even more significant than that due to clouds. The response appears to be a general feature irrespective of the landscape and photosynthetic pathway. The CO2 sink increased with aerosol loading for forest and crop lands, and decreased for grassland. The cause for the difference in response between vegetation types is hypothesized to be canopy architecture.

Received 5 July 2004; accepted 29 September 2004; published 29 October 2004.

Index Terms: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0315 Atmospheric Composition and Structure: Biosphere/atmosphere interactions; 0345 Atmospheric Composition and Structure: Pollution—urban and regional (0305); 1610 Global Change: Atmosphere (0315, 0325); 1615 Global Change: Biogeochemical processes (4805).


Read Full Article (file size: 206703 bytes)    Cited by

Citation: Niyogi, D., et al. (2004), Direct observations of the effects of aerosol loading on net ecosystem CO2 exchanges over different landscapes, Geophys. Res. Lett., 31, L20506, doi:10.1029/2004GL020915.