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GEOPHYSICAL RESEARCH LETTERS, VOL. 33, L22812, doi:10.1029/2006GL027749, 2006

Satellite-observed U.S. power plant NOx emission reductions and their impact on air quality

S.-W. Kim

Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


A. Heckel

Institute of Environmental Physics and Institute of Remote Sensing, University of Bremen, Bremen, Germany


S. A. McKeen

Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


G. J. Frost

Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


E.-Y. Hsie

Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


M. K. Trainer

Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


A. Richter

Institute of Environmental Physics and Institute of Remote Sensing, University of Bremen, Bremen, Germany


J. P. Burrows

Institute of Environmental Physics and Institute of Remote Sensing, University of Bremen, Bremen, Germany


S. E. Peckham

Global Systems Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


G. A. Grell

Global Systems Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA


Abstract

Nitrogen oxide (NOx) emissions resulting from fossil fuel combustion lead to unhealthy levels of near-surface ozone (O3). One of the largest U.S. sources, electric power generation, represented about 25% of the U.S. anthropogenic NOx emissions in 1999. Here we show that space-based instruments observed declining regional NOx levels between 1999 and 2005 in response to the recent implementation of pollution controls by utility companies in the eastern U.S. Satellite-retrieved summertime nitrogen dioxide (NO2) columns and bottom-up emission estimates show larger decreases in the Ohio River Valley, where power plants dominate NOx emissions, than in the northeast U.S. urban corridor. Model simulations predict lower O3 across much of the eastern U.S. in response to these emission reductions.

Received 1 August 2006; accepted 24 October 2006; published 29 November 2006.

Keywords: SCIAMACHY; satellite; power plant; NOx emission.

Index Terms: 0345 Atmospheric Composition and Structure: Pollution: urban and regional (0305, 0478, 4251); 0368 Atmospheric Composition and Structure: Troposphere: constituent transport and chemistry; 0365 Atmospheric Composition and Structure: Troposphere: composition and chemistry.


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Citation: Kim, S.-W., A. Heckel, S. A. McKeen, G. J. Frost, E.-Y. Hsie, M. K. Trainer, A. Richter, J. P. Burrows, S. E. Peckham, and G. A. Grell (2006), Satellite-observed U.S. power plant NOx emission reductions and their impact on air quality, Geophys. Res. Lett., 33, L22812, doi:10.1029/2006GL027749.