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AGU: Global Biogeochemical Cycles

 

Keywords

  • atmospheric CO2
  • transport model
  • synoptic variations

Index Terms

  • Atmospheric Composition and Structure: Troposphere: constituent transport and chemistry
  • Biogeosciences: Biogeochemical cycles, processes, and modeling
  • Atmospheric Processes: Mesoscale meteorology
  • Atmospheric Processes: Boundary layer processes

Abstract

GLOBAL BIOGEOCHEMICAL CYCLES, VOL. 22, GB4013, 16 PP., 2008
doi:10.1029/2007GB003081

TransCom model simulations of hourly atmospheric CO2: Analysis of synoptic-scale variations for the period 2002–2003

P. K. Patra

Frontier Research Center for Global Change, JAMSTEC, Yokohama, Japan

R. M. Law

CSIRO Marine and Atmospheric Research, Aspendale, Victoria, Australia

W. Peters

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Department of Meteorology and Air Quality, Wageningen University and Research Center, Wageningen, Netherlands

C. Rödenbeck

Max-Planck-Institute for Biogeochemistry, Jena, Germany

M. Takigawa

Frontier Research Center for Global Change, JAMSTEC, Yokohama, Japan

C. Aulagnier

Laboratoire des Sciences du Climat et de l'Environnement, IPSL, CEA Saclay, UVSQ, CNRS, Gif Sur Yvette, France

I. Baker

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA

D. J. Bergmann

Lawrence Livermore National Laboratory, Livermore, California, USA

P. Bousquet

Laboratoire des Sciences du Climat et de l'Environnement, IPSL, CEA Saclay, UVSQ, CNRS, Gif Sur Yvette, France

J. Brandt

National Environmental Research Institute, Department of Atmospheric Environment, University of Aarhus, Roskilde, Denmark

L. Bruhwiler

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

P. J. Cameron-Smith

Lawrence Livermore National Laboratory, Livermore, California, USA

J. H. Christensen

National Environmental Research Institute, Department of Atmospheric Environment, University of Aarhus, Roskilde, Denmark

F. Delage

Laboratoire des Sciences du Climat et de l'Environnement, IPSL, CEA Saclay, UVSQ, CNRS, Gif Sur Yvette, France

A. S. Denning

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA

S. Fan

Geophysical Fluid Dynamics Laboratory, NOAA, Princeton, New Jersey, USA

C. Geels

National Environmental Research Institute, Department of Atmospheric Environment, University of Aarhus, Roskilde, Denmark

S. Houweling

Institute for Marine and Atmospheric Research, Utrecht, Netherlands

Netherlands Institute for Space Research, University Utrecht, Utrecht, Netherlands

R. Imasu

Center for Climate System Research, University of Tokyo, Chiba, Japan

U. Karstens

Max-Planck-Institute for Biogeochemistry, Jena, Germany

Max-Planck-Institute for Meteorology, Hamburg, Germany

S. R. Kawa

NASA Goddard Space Flight Center, Greenbelt, Maryland, USA

J. Kleist

Privacy Networks, Fort Collins, Colorado, USA

M. C. Krol

Department of Meteorology and Air Quality, Wageningen University and Research Center, Wageningen, Netherlands

Netherlands Institute for Space Research, University Utrecht, Utrecht, Netherlands

S.-J. Lin

Geophysical Fluid Dynamics Laboratory, NOAA, Princeton, New Jersey, USA

R. Lokupitiya

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA

T. Maki

Atmospheric Environment Division, Japan Meteorological Agency, Tokyo, Japan

S. Maksyutov

Frontier Research Center for Global Change, JAMSTEC, Yokohama, Japan

Center for Global Environmental Research, National Institute for Environmental Studies, Tsukuba, Japan

Y. Niwa

Center for Climate System Research, University of Tokyo, Chiba, Japan

R. Onishi

Earth Simulator Center, JAMSTEC, Yokohama, Japan

N. Parazoo

Department of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA

G. Pieterse

Institute for Marine and Atmospheric Research, Utrecht, Netherlands

Energy Research Centre of the Netherlands, Petten, Netherlands

L. Rivier

Laboratoire des Sciences du Climat et de l'Environnement, IPSL, CEA Saclay, UVSQ, CNRS, Gif Sur Yvette, France

M. Satoh

Frontier Research Center for Global Change, JAMSTEC, Yokohama, Japan

Center for Climate System Research, University of Tokyo, Chiba, Japan

S. Serrar

European Centre for Medium-range Weather Forecasts, Reading, UK

S. Taguchi

National Institute of Advanced Industrial Science and Technology, Tsukuba, Japan

R. Vautard

Laboratoire des Sciences du Climat et de l'Environnement, IPSL, CEA Saclay, UVSQ, CNRS, Gif Sur Yvette, France

A. T. Vermeulen

Energy Research Centre of the Netherlands, Petten, Netherlands

Z. Zhu

Science Systems and Applications Incorporated, Lanham, Maryland, USA

The ability to reliably estimate CO2 fluxes from current in situ atmospheric CO2 measurements and future satellite CO2 measurements is dependent on transport model performance at synoptic and shorter timescales. The TransCom continuous experiment was designed to evaluate the performance of forward transport model simulations at hourly, daily, and synoptic timescales, and we focus on the latter two in this paper. Twenty-five transport models or model variants submitted hourly time series of nine predetermined tracers (seven for CO2) at 280 locations. We extracted synoptic-scale variability from daily averaged CO2 time series using a digital filter and analyzed the results by comparing them to atmospheric measurements at 35 locations. The correlations between modeled and observed synoptic CO2 variabilities were almost always largest with zero time lag and statistically significant for most models and most locations. Generally, the model results using diurnally varying land fluxes were closer to the observations compared to those obtained using monthly mean or daily average fluxes, and winter was often better simulated than summer. Model results at higher spatial resolution compared better with observations, mostly because these models were able to sample closer to the measurement site location. The amplitude and correlation of model-data variability is strongly model and season dependent. Overall similarity in modeled synoptic CO2 variability suggests that the first-order transport mechanisms are fairly well parameterized in the models, and no clear distinction was found between the meteorological analyses in capturing the synoptic-scale dynamics.

Received 6 August 2007; accepted 31 July 2008; published 26 November 2008.

Citation: Patra, P. K., et al. (2008), TransCom model simulations of hourly atmospheric CO2: Analysis of synoptic-scale variations for the period 2002–2003, Global Biogeochem. Cycles, 22, GB4013, doi:10.1029/2007GB003081.

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