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AGU: Geophysical Research Letters

 

Keywords

  • deposition
  • transport
  • nitrogen

Index Terms

  • Atmospheric Composition and Structure: Constituent sources and sinks
  • Atmospheric Composition and Structure: Troposphere: constituent transport and chemistry
  • Global Change: Atmosphere
  • Global Change: Global climate models

Abstract

A multi-model study of the hemispheric transport and deposition of oxidised nitrogen

M. G. Sanderson

Met Office Hadley Centre, Exeter, UK

F. J. Dentener

European Commission, DG JRC, Institute for Environment and Sustainability, Ispra, Italy

A. M. Fiore

NOAA Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey, USA

C. Cuvelier

European Commission, DG JRC, Institute for Environment and Sustainability, Ispra, Italy

T. J. Keating

Office of Policy Analysis and Review, Environmental Protection Agency, Washington, D. C., USA

A. Zuber

Environment Directorate General, European Commission, Brussels, Belgium

C. S. Atherton

Atmospheric Science Division, Lawrence Livermore National Laboratory, Livermore, California, USA

D. J. Bergmann

Atmospheric Science Division, Lawrence Livermore National Laboratory, Livermore, California, USA

T. Diehl

Goddard Earth Science and Technology Center, UMBC, Baltimore, Maryland, USA

R. M. Doherty

School of GeoSciences, University of Edinburgh, Edinburgh, UK

B. N. Duncan

Goddard Earth Science and Technology Center, UMBC, Baltimore, Maryland, USA

P. Hess

National Center for Atmospheric Research, Boulder, Colorado, USA

L. W. Horowitz

NOAA Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey, USA

D. J. Jacob

Atmospheric Chemistry Modelling Group, Harvard University, Cambridge, Massachusetts, USA

J.-E. Jonson

Norwegian Meteorological Institute, Oslo, Norway

J. W. Kaminski

Center for Research in Earth and Space Science, York University, Toronto, Ontario, Canada

A. Lupu

Center for Research in Earth and Space Science, York University, Toronto, Ontario, Canada

I. A. MacKenzie

School of GeoSciences, University of Edinburgh, Edinburgh, UK

E. Mancini

Dipartimento di Fisica, Università L'Aquila, Aquila, Italy

E. Marmer

European Commission, DG JRC, Institute for Environment and Sustainability, Ispra, Italy

R. Park

Atmospheric Chemistry Modelling Group, Harvard University, Cambridge, Massachusetts, USA

G. Pitari

Dipartimento di Fisica, Università L'Aquila, Aquila, Italy

M. J. Prather

Earth System Science, University of California, Irvine, California, USA

K. J. Pringle

Met Office Hadley Centre, Exeter, UK

S. Schroeder

ICG-2, Forschungszentrum-Jülich, Jülich, Germany

M. G. Schultz

ICG-2, Forschungszentrum-Jülich, Jülich, Germany

D. T. Shindell

NASA Goddard Institute for Space Studies and Columbia University, New York, New York, USA

S. Szopa

Laboratoire des Science du Climat et de l'Environment, Gif-sur-Yvette, France

O. Wild

Department of Environmental Science, Lancaster University, Lancaster, UK

P. Wind

Norwegian Meteorological Institute, Oslo, Norway

Fifteen chemistry-transport models are used to quantify, for the first time, the export of oxidised nitrogen (NOy) to and from four regions (Europe, North America, South Asia, and East Asia), and to estimate the uncertainty in the results. Between 12 and 24% of the NOx emitted is exported from each region annually. The strongest impact of each source region on a foreign region is: Europe on East Asia, North America on Europe, South Asia on East Asia, and East Asia on North America. Europe exports the most NOy, and East Asia the least. East Asia receives the most NOy from the other regions. Between 8 and 15% of NOx emitted in each region is transported over distances larger than 1000 km, with 3–10% ultimately deposited over the foreign regions.

Received 18 July 2008; accepted 12 August 2008; published 13 September 2008.

Citation: Sanderson, M. G., et al. (2008), A multi-model study of the hemispheric transport and deposition of oxidised nitrogen, Geophys. Res. Lett., 35, L17815, doi:10.1029/2008GL035389.

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