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AGU: Geophysical Research Letters

 

Keywords

  • methane
  • climate

Index Terms

  • Atmospheric Composition and Structure: Troposphere: composition and chemistry
  • Biogeosciences: Biosphere/atmosphere interactions
  • Biogeosciences: Carbon cycling

Abstract

Observational constraints on recent increases in the atmospheric CH4 burden

E. J. Dlugokencky

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

L. Bruhwiler

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

J. W. C. White

INSTAAR, University of Colorado, Boulder, Colorado, USA

L. K. Emmons

National Center for Atmospheric Research, Boulder, Colorado, USA

P. C. Novelli

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

S. A. Montzka

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

K. A. Masarie

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

P. M. Lang

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

A. M. Crotwell

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

J. B. Miller

NOAA Earth System Research Laboratory, Boulder, Colorado, USA

L. V. Gatti

Divisao de Quimica Ambiental, Laboratorio de Quimica Atmosferica, Insituto de Pesquisas Energéticas e Nucleares, São Paulo, Brazil

Measurements of atmospheric CH4 from air samples collected weekly at 46 remote surface sites show that, after a decade of near-zero growth, globally averaged atmospheric methane increased during 2007 and 2008. During 2007, CH4 increased by 8.3 ± 0.6 ppb. CH4 mole fractions averaged over polar northern latitudes and the Southern Hemisphere increased more than other zonally averaged regions. In 2008, globally averaged CH4 increased by 4.4 ± 0.6 ppb; the largest increase was in the tropics, while polar northern latitudes did not increase. Satellite and in situ CO observations suggest only a minor contribution to increased CH4 from biomass burning. The most likely drivers of the CH4 anomalies observed during 2007 and 2008 are anomalously high temperatures in the Arctic and greater than average precipitation in the tropics. Near-zero CH4 growth in the Arctic during 2008 suggests we have not yet activated strong climate feedbacks from permafrost and CH4 hydrates.

Received 6 July 2009; accepted 18 August 2009; published 17 September 2009.

Citation: Dlugokencky, E. J., et al. (2009), Observational constraints on recent increases in the atmospheric CH4 burden, Geophys. Res. Lett., 36, L18803, doi:10.1029/2009GL039780.

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