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AGU: Geophysical Research Letters

 

Keywords

  • dust
  • absorption
  • photoacoustic

Index Terms

  • Atmospheric Composition and Structure: Aerosols and particles
  • Atmospheric Composition and Structure: Evolution of the atmosphere
  • Atmospheric Composition and Structure: Pollution: urban and regional
  • Atmospheric Composition and Structure: Troposphere: constituent transport and chemistry
  • Atmospheric Composition and Structure: Instruments and techniques

Abstract

GEOPHYSICAL RESEARCH LETTERS, VOL. 36, L24805, 5 PP., 2009
doi:10.1029/2009GL041002

Relative humidity dependence of light absorption by mineral dust after long-range atmospheric transport from the Sahara

Daniel A. Lack

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Cooperative Institute for Research of the Environmental Sciences, University of Colorado, Boulder, Colorado, USA

Patricia K. Quinn

Pacific Marine Environment Laboratory, NOAA, Seattle, Washington, USA

Paola Massoli

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Cooperative Institute for Research of the Environmental Sciences, University of Colorado, Boulder, Colorado, USA

Timothy S. Bates

Pacific Marine Environment Laboratory, NOAA, Seattle, Washington, USA

Derek Coffman

Pacific Marine Environment Laboratory, NOAA, Seattle, Washington, USA

David S. Covert

Atmospheric Sciences Department, University of Washington, Seattle, Washington, USA

Berko Sierau

Atmospheric Sciences Department, University of Washington, Seattle, Washington, USA

Sara Tucker

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Tahllee Baynard

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Cooperative Institute for Research of the Environmental Sciences, University of Colorado, Boulder, Colorado, USA

Edward Lovejoy

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

Daniel M. Murphy

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

A. R. Ravishankara

Earth Systems Research Laboratory, NOAA, Boulder, Colorado, USA

The relative humidity (RH) dependence of light absorption for a Saharan dust-dominated air mass transported to the Gulf of Mexico was measured during the 2006 TexAQS/GoMACCS study using a photo-acoustic absorption spectrometer (PAS). Aerosol absorption was measured at low (25%) and high (73%) RH indicating a 1.5(±0.3) absorption enhancement [f(RHAbs)] under high RH conditions. f(RHAbs) estimates, based on air-mass physical and optical properties and Mie theory modeling, were between 1.2–1.4. Reasons for differences between the measured and modeled f(RHAbs) are discussed. The mass absorption coefficient of the long-range transported dust was calculated to be 0.04(±0.02) m2g−1.

Received 15 September 2009; accepted 17 November 2009; published 19 December 2009.

Citation: Lack, D. A., et al. (2009), Relative humidity dependence of light absorption by mineral dust after long-range atmospheric transport from the Sahara, Geophys. Res. Lett., 36, L24805, doi:10.1029/2009GL041002.

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